Title: Interferometric Characterization of Raman Redistribution Among Perturbed Rydberg States of Barium

D.I. Duncan and R.R. Jones

Abstract:

The evolution of a "dark" wavepacket in Ba is probed using a bound-state interferometric method. The wavepacket is created by photoionizing the 5d7d component of a perturbed Rydberg state having predominantly 6snd character and thereby, redistributing population to neighboring states. Information on which Rydberg-Rydberg transitions dominate the transfer of population to each state is obtained. A closed form expression for the observed strong-field interferograms is developed for the limit of very short pulses.

Status: Published, Phys. Rev. A 53, 4338 (1996)
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